What's Up With Chisei?
One of the most commonly misunderstood, misinterpreted, or just plain missed things in the canon is the question of what, exactly, is going on with Chisei.
Which is to say: why is his age in quotes, is he being serious when he said he died, and what is going on?
The short answer is:
Kuzuryu Chisei is dead, and the Chisei that we see interacting with characters in the present in the canon is a phantom illusion being manifested by Haruomi.
So what does that mean?
With the above evidence that Chisei is dead, the general working understanding is that the Chisei we see interacting with the rest of the cast is a metal phantom created by Haruomi -- inspired by Kanata doing the same to create a phantom Nayuta -- based on Chisei as he was ten years ago at age 28. Hence, his age is in quotation marks.
Haruomi's aged appearance in the present is loosely implied to be the result of premature aging thanks to habitual phantometal use, and it is possible that his own younger appearance is also a phantom created for the purpose of public appearances/performances.
When Chisei appears in LIVE part 4, he is assumed to be an illusion. Haruomi, unlike Kanata, appears to be aware that he is manifesing an illusion of a dead person, but is keeping the illusion up for his own undisclosed reasons.
We know from phantom Nayuta that metal phantoms are capable of acting and speaking indepenently from the person generating them, and are corporeal enough to manipulate physical objects (see: the Nayuta phantom in the LOVE dramas).
So, yes, when Chisei says "because I up and died", you should take it at face value.
But that said...
... so I wrote all this a while ago, and now this is all kind of a moot point, because the anime basically outright said that Chisei is dead.
So, hey, I was right, at least!
Whether you take the anime as canon or not is your own cross to bear. Many parts of the anime, especially (unfortunately) the parts from which we draw this information, are incompatible with the drama track canon, but if you choose to accept it as canon, then it resolves this ambiguity entirely.
The anime features a phantom Buraikan created by Alter Trigger for the purposes of the first Paradox Live; if we attempt to fold this information into the drama canon, we can assume that Haruomi continues to create the phantom Chisei on his own. Indeed, the special voice dramas included as a bonus from the full BD set confirmed that Haruomi was specifically inspired by Kanata's use of phantoms to create a Chisei phantom.
Visuals at the beginning of episode 11 seem to confirm that it was phantometal erosion that killed him. A line from the Alter Trigger scientist may seem to contradict this, thanks to the way the official subtitles say "the same way Yasha died" as he's firing a gun at Shura; but, based on the actual line in Japanese, I believe this is probably meant to mean "and you're going to die, too", and is not a remark on how Chisei died.
Again: unfortunately, there are many things about the anime that are incompatible with canon, but the Buraikan information does mostly track with and confirm what was hinted at in the drama tracks, because Buraikan are basically the only group that made it out of the anime without their story and characterization being put through a meat grinder, lol.